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Great for kids (young and old).

Refrederator, the free daily cartoon podcast – a classic cartoon every day (Bugs Bunny, Mighty Mouse, Daffy Duck, Betty Boop, Porky Pig, Donald Duck and Felix the Cat, etc). Simply add http://refrederator.com/rss to your device via Zune Software.

Nick Jr. Simply pick your podcast, preview, and then copy RSS link into Zune Software. Currrently available are Dora the Explorer, Go Diego, Go and Blues Clues

Cartoon Network also has available podcasts. Episodes vary from week to week. Again, simply enter RSS feed into your Zune Software.

Discovery channel

http://www.discovery.com/radio/xml/discovery_video.xml

To add a podcast: In Zune Software, select device, select podcasts , enter RSS URL and hit subscribe. You can edit the settings to increase/decrease the number of episodes you want to keep on your device