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You could try deselecting email as a sync option, syncing and then putting email back on as an option. Also, are you sure haven't dragged your inbox to a funny place in the folder structure of Outlook on your PC? If the folder isn't in the normal order that can be problematic. Also, you could try adjusting the size of files/attachments you want synced onto your system or try saving the messages on a memory card instead of on the device itself.
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