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Are you using multiple Outlook profiles like the error message suggests? If you, it should be prompting you for the right profile when you synch (and also when you start Outlook). Try cradling the PDA without Outlook running (if Outlook is already running with the wrong profile you might get a message like this).
Or if your Outlook profile is password-protected like it suggests, remove the password (I'm not sure where that is set).
You can manage Outlook profiles by going to Control Panel -> Mail, and clickng the Show Profiles... button. Looking at the settings (including data file locations) for each profile might give you some clues.
If none of the above helps, try deleting your ActiveSync relationships (is that the right word? I'm still asleep). Also try deleting all Outlook profiles. Then set things up again. Deleting Outlook profiles won't destroy your appointments etc., but you will have to find the right PST file and your email server settings in order to set up the new profile.
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